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Dehydrogenation of liquid fuel in microchannel catalytic reactor

United States Patent

August 3, 2010
View the Complete Patent at the US Patent & Trademark Office
The present invention is an improved process for the storage and delivery of hydrogen by the reversible hydrogenation/dehydrogenation of an organic compound wherein the organic compound is initially in its hydrogenated state. The improvement in the route to generating hydrogen is in the dehydrogenation step and recovery of the dehydrogenated organic compound resides in the following steps: introducing a hydrogenated organic compound to a microchannel reactor incorporating a dehydrogenation catalyst; effecting dehydrogenation of said hydrogenated organic compound under conditions whereby said hydrogenated organic compound is present as a liquid phase; generating a reaction product comprised of a liquid phase dehydrogenated organic compound and gaseous hydrogen; separating the liquid phase dehydrogenated organic compound from gaseous hydrogen; and, recovering the hydrogen and liquid phase dehydrogenated organic compound.
Toseland; Bernard Allen (Coopersburg, PA), Pez; Guido Peter (Allentown, PA), Puri; Pushpinder Singh (Emmaus, PA)
Air Products & Chemicals, Inc. (Allentown, PA)
12/ 211,585
September 16, 2008
STATEMENT REGARDING FEDERALLY SPONSORED RESEARCH OR DEVELOPMENT This invention was made with government support under Contract Number DE-FG36-05GO15015 between Air Products and Chemicals, Inc. and the U.S. Department of Energy. The Government has certain rights to this invention.