In various embodiments, the present disclosure provides methods of forming graphene films by: (1) depositing a non-gaseous carbon source onto a catalyst surface; (2) exposing the non-gaseous carbon source to at least one gas with a flow rate; and (3) initiating the conversion of the non-gaseous carbon source to the graphene film, where the thickness of the graphene film is controllable by the gas flow rate. Additional embodiments of the present disclosure pertain to graphene films made in accordance with the methods of the present disclosure.
STATEMENT REGARDING FEDERALLY SPONSORED RESEARCH
This invention was made with government support under Sandia National Laboratory Grant No. 1100745, awarded by the U.S. Department of Energy; Office of Naval Research Grant No. N00014-09-1-1066, awarded by the U.S. Department of Defense; and Air Force Office of Scientific Research Grant No. FA 9550-09-1-0581, awarded by the U.S. Department of Defense. The government has certain rights in the invention.