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Method of CO.sub.2 removal from a gasesous stream at reduced temperature

United States Patent

November 18, 2014
View the Complete Patent at the US Patent & Trademark Office
National Energy Technology Laboratory - Visit the Technology Transfer Website
A method for the removal of H.sub.2O and CO.sub.2 from a gaseous stream comprising H.sub.2O and CO.sub.2, such as a flue gas. The method initially utilizes an H.sub.2O removal sorbent to remove some portion of the H.sub.2O, producing a dry gaseous stream and a wet H.sub.2O removal sorbent. The dry gaseous stream is subsequently contacted with a CO.sub.2 removal sorbent to remove some portion of the CO.sub.2, generating a dry CO.sub.2 reduced stream and a loaded CO.sub.2 removal sorbent. The loaded CO.sub.2 removal sorbent is subsequently heated to produce a heated CO.sub.2 stream. The wet H.sub.2O removal sorbent and the dry CO.sub.2 reduced stream are contacted in a first regeneration stage, generating a partially regenerated H.sub.2O removal sorbent, and the partially regenerated H.sub.2O removal sorbent and the heated CO.sub.2 stream are subsequently contacted in a second regeneration stage. The first and second stage regeneration typically act to retain an initial monolayer of moisture on the various removal sorbents and only remove moisture layers bound to the initial monolayer, allowing for relatively low temperature and pressure operation. Generally the applicable H.sub.2O sorption/desorption processes may be conducted at temperatures less than about C. and pressures less than 1.5 atmospheres, with certain operations conducted at temperatures less than about C.
Fisher; James C. (Morgantown, WV), Siriwardane; Ranjani V. (Morgantown, WV), Berry; David A. (Mount Morris, PA), Richards; George A. (Morgantown, WV)
U.S. Department of Energy (Washington, DC)
14/ 022,708
September 10, 2013
GOVERNMENT INTERESTS The United States Government has rights in this invention pursuant to the employer-employee relationship of the Government to the inventors as U.S. Department of Energy employees and site-support contractors at the National Energy Technology Laboratory.