A process for the production of a reaction product including a carbon containing compound. The process includes providing a film of a fuel source including at least one organic compound on a wall of a reactor, contacting the fuel source with a source of oxygen, forming a vaporized mixture of fuel and oxygen, and contacting the vaporized mixture of fuel and oxygen with a catalyst under conditions effective to produce a reaction product including a carbon containing compound. Preferred products include .alpha.-olefins and synthesis gas. A preferred catalyst is a supported metal catalyst, preferably including rhodium, platinum, and mixtures thereof.
STATEMENT OF GOVERNMENT RIGHTS
The present invention was made with support by the ARL Collaborative Technology Alliance in Power and Energy, Cooperative Agreement No. DAAD19-01-2-0010; U.S. Army Grant #DAAD19-00-R-0005; and Department of Energy Grant #DE-FC05-97OR22579. The United States government has certain rights in the invention.